Summary Sources:
1. Bengo - https://www.citypopulation.de/en/angola/admin/18__bengo/ - Majority Native
2. Benguela - http://www.citypopulation.de/en/angola/admin/09__benguela/ - Majority Native
3. Bié - https://www.citypopulation.de/en/angola/admin/11__bi%C3%A9/ - Not Majority Native but almost
4. Cabinda - http://www.citypopulation.de/en/angola/admin/01__cabinda/ - Majority Native
5. Cuando Cubango - https://www.citypopulation.de/en/angola/admin/13__cuando_cubango/ - Not Majority Native but almost
6. Cuanza Norte - https://www.citypopulation.de/en/angola/admin/05__cuanza_norte/ - Majority Native
7. Cuanza Sul - https://www.citypopulation.de/en/angola/admin/06__cuanza_sul/ - Majority Native
8. Cunene - https://www.citypopulation.de/en/angola/communes/admin/16__cunene/ - Not Majority
9. Huambo - https://www.citypopulation.de/en/angola/admin/10__huambo/ - Not Majority Native but almost
10. Huíla -http://www.citypopulation.de/en/angola/admin/15__hu%C3%ADla/ - Majority Native
11. Luanda - https://www.citypopulation.de/en/angola/admin/04__luanda/ - Majority Native
12. Lunda Norte - https://www.citypopulation.de/en/angola/admin/08__lunda_norte/ - Not Majority Native but almost
13. Lunda Sul - https://www.citypopulation.de/en/angola/admin/17__lunda_sul/ - Not Majority Native but almost
14. Malanje - https://www.citypopulation.de/en/angola/admin/07__malanje/ - Majority Native
15. Moxico - https://www.citypopulation.de/en/angola/admin/12__moxico/ - Not Majority
16. Namibe - https://www.citypopulation.de/en/angola/admin/14__namibe/ - Majority Native
17. Uíge - http://www.citypopulation.de/en/angola/admin/03__u%C3%ADge/ - Majority Native
18. Zaire - https://www.citypopulation.de/en/angola/admin/02__zaire/ - Not Majority
Results: 11 out of 18 provinces are majority native Portuguese speaking.
5 out of 18 provinces are almost majority native Portuguese speaking.
2 out of 18 provinces are not close to being majority native Portuguese speaking.
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